Another scene with James Gandolfini which in my opinion, supersedes any of them is the beating he threw to Patricia Arquette in the movie True Romance...which is the scene in which David Chase made his decision to cast Gandolfini as Tony Soprano. Also, the scene where he beat the shit out of Coco at his restaurant in Little Italy when he made him bite down on the fireplace.

The final episode of the most recent season (4) of Boardwalk Empire, where Eli beat to death the FBI agent.